Aharonov-Bohm phase as quantum gate in two-electron charge qubits

We analyze the singlet-triplet splitting on a planar array of quantum dots coupled capacitively to a set of external voltage gates. The system is modelled using an extended Hubbard Hamiltonian keeping two excess electrons on the array. The voltage dependence of the low-energy singlet and triplet states is analyzed using the Feshbach formalism. The formation of a well decoupled two-level system in the ground state is shown to rely on the fact of having two particles in the system. Coherent operation of the array is studied with respect to single quantum bit operations. One quantum gate is implemented via voltage controls, while for the necessary second quantum gate, a uniform external magnetic field is introduced. The Aharonov-Bohm phases on the closed loop tunnel connections in the array are used to effectively suppress the tunneling, despite a constant tunneling amplitude in the structure. This allows one to completely stall the qubit in any arbitrary quantum superposition, providing full control of this interesting quantum system.Comment: 6 pages, 5 figures (submitted to PRB

Potential landscapes and induced charges near metallic islands in three dimensions

We calculate electrostatic potential landscapes for an external probe charge in the presence of a set of metallic islands. Our numerical calculation in three dimensions (3D)uses an efficient grid relaxation technique. The well-known relaxation algorithm for solving the Poisson equation in two dimensions is generalized to 3D. In addition,all charges on the system, free as well as induced charges,are determined accurately and self-consistently to satisfy the desired boundary conditions. This allows the straightforward calculation of the potential on the outer boundary using the free space electrostatic Green's function,as well as the calculation of the entire capacitance matrix of the system. Physically interesting examples of nanoscale systems are presented and analyzed.Comment: 6 pages, 6 figures, submitted to PR

Sum-rule Conserving Spectral Functions from the Numerical Renormalization Group

We show how spectral functions for quantum impurity models can be calculated very accurately using a complete set of ``discarded'' numerical renormalization group eigenstates, recently introduced by Anders and Schiller. The only approximation is to judiciously exploit energy scale separation. Our derivation avoids both the overcounting ambiguities and the single-shell approximation for the equilibrium density matrix prevalent in current methods, ensuring that relevant sum rules hold rigorously and spectral features at energies below the temperature can be described accurately.Comment: 4 pages + 1 page appendix, 2 figure

Matrix product state approach for a two-lead, multi-level Anderson impurity model

We exploit the common mathematical structure of the numerical renormalization group and the density matrix renormalization group, namely, matrix product states, to implement an efficient numerical treatment of a two-lead, multi-level Anderson impurity model. By adopting a star-like geometry, where each species (spin and lead) of conduction electrons is described by its own Wilson chain, instead of using a single Wilson chain for all species together, we achieve a very significant reduction in the numerical resources required to obtain reliable results. We illustrate the power of this approach by calculating ground state properties of a four-level quantum dot coupled to two leads. The success of this proof-of-principle calculation suggests that the star geometry constitutes a promising strategy for future calculations the ground state properties of multi-band, multi-level quantum impurity models. Moreover, we show that it is possible to find an "optimal" chain basis, obtained via a unitary transformation (acting only on the index distinguishing different Wilson chains), in which degrees of freedom on different Wilson chains become effectively decoupled from each other further out on the Wilson chains. This basis turns out to also diagonalize the model's chain-to-chain scattering matrix. We demonstrate this for a spinless two-lead model, presenting DMRG-results for the mutual information between two sites located far apart on different Wilson chains, and NRG results with respect to the scattering matrix.Comment: extended version, 11 pages, 12 figure

Charge qubits and limitations of electrostatic quantum gates

We investigate the characteristics of purely electrostatic interactions with external gates in constructing full single qubit manipulations. The quantum bit is naturally encoded in the spatial wave function of the electron system. Single-electron{transistor arrays based on quantum dots or insulating interfaces typically allow for electrostatic controls where the inter-island tunneling is considered constant, e.g. determined by the thickness of an insulating layer. A representative array of 3x3 quantum dots with two mobile electrons is analyzed using a Hubbard Hamiltonian and a capacitance matrix formalism. Our study shows that it is easy to realize the first quantum gate for single qubit operations, but that a second quantum gate only comes at the cost of compromising the low-energy two-level system needed to encode the qubit. We use perturbative arguments and the Feshbach formalism to show that the compromising of the two-level system is a rather general feature for electrostatically interacting qubits and is not just related to the specific details of the system chosen. We show further that full implementation requires tunable tunneling or external magnetic fields.Comment: 7 pages, 5 figures, submitted to PR

Non-Fermi liquid behavior in transport through Co doped Au chains

We calculate the conductance as a function of temperature $G(T)$ through Au monoatomic chains containing one Co atom as a magnetic impurity, and connected to two conducting leads with a 4-fold symmetry axis. Using the information derived from {\it ab initio} calculations, we construct an effective model \Heff that hybridizes a 3d$^7$ quadruplet at the Co site with two 3d$^8$ triplets through the hopping of 5d$_{xz}$ and 5d$_{yz}$ electrons of Au. The quadruplet is split by spin anisotropy due to spin-orbit coupling. Solving \Heff with the numerical renormalization group (NRG) % Wb: reverted my own change we find that at low temperatures $G(T)=a-b \sqrt{T}$ and the ground state impurity entropy is $\ln(2)/2$, a behavior similar to the two-channel Kondo model. Stretching the chain leads to a non Kondo phase, with the physics of the underscreened Kondo model at the quantum critical point.Comment: Accepted in Physical Review Letter

Variational matrix product state approach to quantum impurity models

We present a unified framework for renormalization group methods, including Wilson's numerical renormalization group (NRG) and White's density-matrix renormalization group (DMRG), within the language of matrix product states. This allows improvements over Wilson's NRG for quantum impurity models, as we illustrate for the one-channel Kondo model. Moreover, we use a variational method for evaluating Green's functions. The proposed method is more flexible in its description of spectral properties at finite frequencies, opening the way to time-dependent, out-of-equilibrium impurity problems. It also substantially improves computational efficiency for one-channel impurity problems, suggesting potentially \emph{linear} scaling of complexity for $n$-channel problems.Comment: revised version with application to Kondo model at large magnetic field (5 pages, 2 figures